On the forces acting on a small particle in an acoustical field in a viscous fluid

We calculate the acoustic radiation force from an ultrasound wave on a compressible, spherical particle suspended in a viscous fluid. Using Prandtl--Schlichting boundary-layer theory, we include the kinematic viscosity of the solvent and derive an analytical expression for the resulting radiation force, which is valid for any particle radius and boundary-layer thickness provided that both of these length scales are much smaller than the wavelength of the ultrasound wave (mm in water at MHz frequencies). The acoustophoretic response of suspended microparticles is predicted and analyzed using parameter values typically employed in microchannel acoustophoresis.Comment: 12 pages, 4 figure

Scaling behavior of optimally structured catalytic microfluidic reactors

In this study of catalytic microfluidic reactors we show that, when optimally structured, these reactors share underlying scaling properties. The scaling is predicted theoretically and verified numerically. Furthermore, we show how to increase the reaction rate significantly by distributing the active porous material within the reactor using a high-level implementation of topology optimization.Comment: 4 pages, 5 eps figure

Localized plasmons in point contacts

Using a hydrodynamic model of the electron fluid in a point contact geometry we show that localized plasmons are likely to exist near the constriction. We attempt to relate these plasmons with the recent experimental observation of deviations of the quantum point contact conductance from ideal integer quantization. As a function of temperature this deviation exhibits an activated behavior, exp(-T_a/T), with a density dependent activation temperature T_a of the order of 2 K. We suggest that T_a can be identified with the energy needed to excite localized plasmons, and we discuss the conductance deviations in terms of a simple theoretical model involving quasiparticle lifetime broadening due to coupling to the localized plasmons.Comment: 5 pages (Latex) including 1 postscript figur

A sharp-interface model of electrodeposition and ramified growth

We present a sharp-interface model of two-dimensional ramified growth during quasi-steady electrodeposition. Our model differs from previous modeling methods in that it includes the important effects of extended space-charge regions and nonlinear electrode reactions. The model is validated by comparing its behavior in the initial stage with the predictions of a linear stability analysis.Comment: RevTex, 14 pages, 12 eps figure

Acoustic interaction forces between small particles in an ideal fluid

We present a theoretical expression for the acoustic interaction force between small spherical particles suspended in an ideal fluid exposed to an external acoustic wave. The acoustic interaction force is the part of the acoustic radiation force on one given particle involving the scattered waves from the other particles. The particles, either compressible liquid droplets or elastic microspheres, are considered to be much smaller than the acoustic wavelength. In this so-called Rayleigh limit, the acoustic interaction forces between the particles are well approximated by gradients of pair-interaction potentials with no restriction on the inter-particle distance. The theory is applied to studies of the acoustic interaction force on a particle suspension in either standing or traveling plane waves. The results show aggregation regions along the wave propagation direction, while particles may attract or repel each other in the transverse direction. In addition, a mean-field approximation is developed to describe the acoustic interaction force in an emulsion of oil droplets in water.Comment: 11 pages, 5 eps figures, RevTex 4.

Acoustic Tweezing and Patterning of Concentration Fields in Microfluidics

We demonstrate theoretically that acoustic forces acting on inhomogeneous fluids can be used to pattern and manipulate solute concentration fields into spatio-temporally controllable configurations stabilized against gravity. A theoretical framework describing the dynamics of concentration fields that weakly perturb the fluid density and speed of sound is presented and applied to study manipulation of concentration fields in rectangular-channel acoustic eigenmodes and in Bessel-function acoustic vortices. In the first example, methods to obtain horizontal and vertical multi-layer stratification of the concentration field at the end of a flow-through channel are presented. In the second example, we demonstrate acoustic tweezing and spatio-temporal manipulation of a local high-concentration region in a lower-concentration medium, thereby extending the realm of acoustic tweezing to include concentration fields.Comment: Revtex, 9 pages, 5 eps figure

Forces acting on a small particle in an acoustical field in a thermoviscous fluid

We present a theoretical analysis of the acoustic radiation force on a single small particle, either a thermoviscous fluid droplet or a thermoelastic solid particle, suspended in a viscous and heat-conducting fluid medium. Our analysis places no restrictions on the length scales of the viscous and thermal boundary layer thicknesses $\delta_\mathrm{s}$ and $\delta_\mathrm{t}$ relative to the particle radius $a$, but it assumes the particle to be small in comparison to the acoustic wavelength $\lambda$. This is the limit relevant to scattering of sound and ultrasound waves from micrometer-sized particles. For particles of size comparable to or smaller than the boundary layers, the thermoviscous theory leads to profound consequences for the acoustic radiation force. Not only do we predict forces orders of magnitude larger than expected from ideal-fluid theory, but for certain relevant choices of materials, we also find a sign change in the acoustic radiation force on different-sized but otherwise identical particles. This phenomenon may possibly be exploited in handling of submicrometer-sized particles such as bacteria and vira in lab-on-a-chip systems.Comment: Revtex, 23 pages, 4 eps figure

Concentration polarization, surface currents, and bulk advection in a microchannel

We present a comprehensive analysis of salt transport and overlimiting currents in a microchannel during concentration polarization. We have carried out full numerical simulations of the coupled Poisson-Nernst-Planck-Stokes problem governing the transport and rationalized the behaviour of the system. A remarkable outcome of the investigations is the discovery of strong couplings between bulk advection and the surface current; without a surface current, bulk advection is strongly suppressed. The numerical simulations are supplemented by analytical models valid in the long channel limit as well as in the limit of negligible surface charge. By including the effects of diffusion and advection in the diffuse part of the electric double layers, we extend a recently published analytical model of overlimiting current due to surface conduction.Comment: 15 pages, 11 figures, Revtex 4.

The Spectrum of the two dimensional Hubbard model at low filling

Using group theoretical and numerical methods we have calculated the exact energy spectrum of the two-dimensional Hubbard model on square lattices with four electrons for a wide range of the interaction strength. All known symmetries, i.e.\ the full space group symmetry, the SU(2) spin symmetry, and, in case of a bipartite lattice, the SU(2) pseudospin symmetry, have been taken explicitly into account. But, quite remarkably, a large amount of residual degeneracies remains giving strong evidence for the existence of a yet unknown symmetry. The level spacing distribution and the spectral rigidity are found to be in close to but not exact agreement with random matrix theory. In contrast, the level velocity correlation function presents an unexpected exponential decay qualitatively different from random matrix behavior.Comment: 4 pages, latex (revtex), 3 uuencoded postscript figure